Cavity-induced anti-correlated photon emission rates of a single ion

We report on the alteration of photon emission properties of a single trapped ion coupled to a high finesse optical fiber cavity. We show that the vacuum field of the cavity can simultaneously affect the emissions in both the infrared (IR) and ultraviolet (UV) branches of the $\Lambda-$type level system of $^{40}\mathrm{Ca}^+$ despite the cavity coupling only to the IR transition. The cavity induces strong emission in the IR transition through the Purcell effect resulting in a simultaneous suppression of the UV fluorescence. The measured suppression of this fluorescence is as large as 66% compared with the case without the cavity. Through analysis of the measurement results, we have obtained an ion-cavity coupling of $\bar{g}_0 = 2\pi\cdot (5.3 \pm 0.1)$ MHz, the largest ever reported so far for a single ion in the IR domain.