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arxiv: 1712.09398 · v1 · pith:2VOTJYTKnew · submitted 2017-12-26 · ⚛️ physics.optics · quant-ph

Life-time and line-width of individual quantum dots interfaced with graphene

classification ⚛️ physics.optics quant-ph
keywords life-timeinterfacedconductivedotsfluorescencegrapheneindividualline-width
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We report on the luminescence's life-time and line-width from an array of individual quantum dots; these were interfaced with graphene surface guides or dispersed on a metal film. Our results are consistent with screening by charge carriers. Fluorescence quenching is typically mentioned as a sign that chromophores are interfacing a conductive surface; we found that QD interfaced with conductive layers exhibited shorter life-time and line-broadening but not necessarily fluorescence quenching as the latter may be impacted by molecular concentration, reflectivity and conductor imperfections. We also comment on selective life-time measurements, which, we postulate depend on the specifics of the local density-of-states involved.

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