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arxiv: 1801.00426 · v1 · pith:W7ET66ZBnew · submitted 2018-01-01 · ❄️ cond-mat.str-el · cond-mat.mes-hall

Chiral spin texture in the charge-density-wave phase of the correlated metallic Pb/Si(111) monolayer

classification ❄️ cond-mat.str-el cond-mat.mes-hall
keywords correlatedfermiinteractionlargelow-temperaturemonolayerphaserelativistic
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We investigate the 1/3 monolayer $\alpha$-Pb/Si(111) surface by scanning tunneling spectroscopy (STS) and fully relativistic first-principles calculations. We study both the high-temperature $\sqrt{3}\times\sqrt{3}$ and low-temperature $3\times 3$ reconstructions and show that, in both phases, the spin-orbit interaction leads to an energy splitting as large as $25\%$ of the valence-band bandwidth. Relativistic effects, electronic correlations and Pb-substrate interaction cooperate to stabilize a correlated low-temperature paramagnetic phase with well-developed lower and upper Hubbard bands coexisting with $3\times3$ periodicity. By comparing the Fourier transform of STS conductance maps at the Fermi level with calculated quasiparticle interference from non-magnetic impurities, we demonstrate the occurrence of two large hexagonal Fermi sheets with in-plane spin polarizations and opposite helicities.

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