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Vanadium trimers randomly aligned along the c-axis direction in layered LiVO2

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arxiv 1910.01337 v1 pith:KBZ6NON2 submitted 2019-10-03 cond-mat.str-el cond-mat.mtrl-sci

K. Kojima , N. Katayama , S. Tamura , M. Shiomi , H. Sawa This is my paper · ORCID
classification cond-mat.str-elcond-mat.mtrl-sci
keywords livo2trimersvanadiumalongc-axisdirectionalignedlayered
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Herein, we discuss the identification of vanadium trimers in layered LiVO2 and its sulfide analog of LiVS2 with two-dimensional triangular lattices. Our comprehensive structural studies using synchrotron X-ray diffraction experiments clarified that vanadium trimers are randomly aligned along the c-axis direction in LiVO2, while the long-range ordering of vanadium trimers along the c-axis direction appears in LiVS2. Our results solve the longstanding issue of cluster patterns in LiVO2 and provide an experimental basis for identifying the mechanism of trimer formation.

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