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Field-orientation-dependent magnetic phases in GdRu$_2$Si$_2$ probed with muon-spin spectroscopy

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arxiv 2403.09431 v3 pith:GGDU52N4 submitted 2024-03-14 cond-mat.str-el

classification cond-mat.str-el
keywords muonappliedmagneticphasesgdrucrystallographicdistinctevidence
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abstract

Centrosymmetric GdRu$_2$Si$_2$ exhibits a variety of multi-Q magnetic states as a function of temperature and applied magnetic field, including a square skyrmion-lattice phase. The material's behavior is strongly dependent on the direction of the applied field, with different phase diagrams resulting for fields applied parallel or perpendicular to the crystallographic $c$ axis. Here, we present the results of muon-spin relaxation ($\mu^+$SR) measurements on single crystals of GdRu$_2$Si$_2$. Our analysis is based on the computation of muon stopping sites and consideration of zero-point motion effects, allowing direct comparison with the underlying spin textures in the material. The muon site is confirmed experimentally, using angle-dependent measurements of the muon Knight shift. Using transverse-field $\mu^+$SR with fields applied along either the [001] or [100] crystallographic directions, we distinguish between the magnetic phases in this system via their distinct muon response, providing additional evidence for the skyrmion and meron-lattice phases, while also suggesting the existence of RKKY-driven muon hyperfine coupling. Zero-field $\mu^+$SR provides clear evidence for a transition between two distinct magnetically-ordered phases at 39 K.

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  1. A Magnon Band Analysis of GdRu2Si2 in the Field-Polarized State

    cond-mat.str-el 2025-01 conditional novelty 6.0 of 10

    Inelastic neutron scattering in the field-polarized state of GdRu2Si2 yields a magnon dispersion fitted by bilinear Heisenberg exchange interactions J1 through J8, with no sign of higher-order or anisotropic terms.

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