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arxiv: 2503.15744 · v2 · pith:NSFIFNWE · submitted 2025-03-19 · cond-mat.soft

Transient Chirality in the Gelation of Adhesive Spinner Monolayers

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classification cond-mat.soft
keywords chiralitygelationadhesivemonolayersspinneractiveactivityaggregation
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Active systems of self-rotating elements inherently exhibit chirality, making them of fundamental interest due to parity violation. Using large-scale hydrodynamic simulations, we investigate the gelation of adhesive spinners confined to quasi-2D monolayers at low Reynolds numbers. Unlike the coarsening dynamics of passive colloids, spinner gelation follows a different pathway, displaying structural chirality during the early stages of aggregation. However, this chirality dissipates upon dynamical arrest, resulting in a final gel structure that resembles a conventional colloidal gel. As a result, we find no sign of odd mechanical responses. Nonetheless, the elastic modulus and gelation time remain tunable through spinning activity, providing a new avenue for the bottom-up design of programmable soft materials.

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