Robust and High-Fidelity Controlled Two-Qubit Gates via Asymmetric Parallel Resonant Excitation
Pith reviewed 2026-05-10 17:47 UTC · model grok-4.3
The pith
Asymmetric resonant excitation enables robust controlled two-qubit gates with over 99% fidelity despite spectral inhomogeneity.
A machine-rendered reading of the paper's core claim, the machinery that carries it, and where it could break.
Core claim
The authors demonstrate that asymmetric resonant driving combined with pulse engineering produces arbitrary controlled two-qubit gates that remain decoupled and robust to detuning, achieving simulated fidelities exceeding 99% over a 170 kHz range with off-resonant excitation held below 0.2% in rare-earth-ion ensemble qubits.
What carries the argument
Asymmetric parallel resonant excitation with tailored pulse sequences, which maintains resonance while decoupling the two qubits' dynamics under dipole-dipole interaction.
If this is right
- Gate fidelities exceed 99% across a 170 kHz detuning range.
- Off-resonant excitation stays below 0.2% for the chosen parameters.
- The scheme supports arbitrary controlled two-qubit gates rather than only specific rotations.
- The approach reduces sensitivity to frequency calibration errors compared with detuned-pulse methods.
Where Pith is reading between the lines
- Similar resonant asymmetric driving may apply to other platforms dominated by dipole or van der Waals interactions.
- The pulse-engineering step could be adapted to compensate for additional known noise sources once they are characterized.
- If experimentally confirmed, the method lowers the precision required for frequency stabilization in large-scale ion or defect arrays.
Load-bearing premise
Numerical simulations faithfully represent the actual dipole-dipole couplings, pulse distortions, and decoherence mechanisms present in the physical rare-earth-ion system.
What would settle it
Laboratory implementation of the proposed pulse sequence on a rare-earth ion crystal, followed by measurement of controlled-gate fidelity as a continuous function of laser detuning to verify whether fidelity stays above 99% throughout the 170 kHz window.
read the original abstract
Implementing high-fidelity controlled two-qubit gates in dipole-dipole interacting systems, such as rare-earth-ion crystals, in hindered by spectral inhomogeneity and weak coupling. Existing method often rely on detuned pulses, making them susceptible to frequency errors and AC Stark shifts. We propose a robust resonant scheme for arbitrary controlled two-qubit gates that utilizes asymmetric excitation and pulse engineering to achieve decoupled, parallel qubit control. Simulations on rare-earth-ion ensemble qubits demonstrate gate fidelities exceeding 99% within a 170 kHz detuning range with off-resonant excitation below 0.2%. This approach offers a robust, scalable route for quantum computing in spectrally crowded systems.
Editorial analysis
A structured set of objections, weighed in public.
Referee Report
Summary. The manuscript proposes a resonant scheme for controlled two-qubit gates in dipole-dipole coupled systems with spectral inhomogeneity (e.g., rare-earth-ion ensembles). It employs asymmetric parallel resonant excitation and pulse engineering to achieve decoupled control, claiming via numerical simulations gate fidelities exceeding 99% over a 170 kHz detuning window with off-resonant excitation below 0.2%. The approach is positioned as more robust than detuned-pulse methods against frequency errors and AC Stark shifts.
Significance. If the simulation results hold under realistic conditions, the scheme would offer a practical route to high-fidelity two-qubit operations in ensemble-based platforms where inhomogeneous broadening and weak couplings have limited prior methods. The reported robustness range and low leakage are potentially enabling for scalable quantum computing in spectrally crowded systems.
major comments (2)
- [Simulation/results section] The central claim of >99% fidelity within a 170 kHz detuning range (abstract and results) rests entirely on numerical simulations, yet the manuscript provides no explicit description of the modeled Hamiltonian, including the specific form and strength of dipole-dipole interactions, spectral diffusion rates, or pulse-shape implementation details. Without these, the 170 kHz robustness window and 0.2% off-resonant bound cannot be independently validated or reproduced.
- [Methods/simulation details] The weakest modeling assumption—that the simulated dynamics accurately capture collective effects, AC Stark shifts from off-resonant excitation, and all relevant decoherence channels—is not tested against experimental benchmarks or parameter sweeps. Any systematic underestimation of these terms would directly invalidate the reported fidelity and detuning tolerance.
minor comments (1)
- [Theory section] Notation for the asymmetric pulse parameters and the definition of the detuning range should be clarified with explicit equations to allow readers to connect the scheme to the simulation results.
Simulated Author's Rebuttal
We thank the referee for their careful and constructive review of our manuscript. The comments highlight important aspects of reproducibility and validation that we have addressed through revisions to the simulation details and additional analysis.
read point-by-point responses
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Referee: [Simulation/results section] The central claim of >99% fidelity within a 170 kHz detuning range (abstract and results) rests entirely on numerical simulations, yet the manuscript provides no explicit description of the modeled Hamiltonian, including the specific form and strength of dipole-dipole interactions, spectral diffusion rates, or pulse-shape implementation details. Without these, the 170 kHz robustness window and 0.2% off-resonant bound cannot be independently validated or reproduced.
Authors: We agree that the original manuscript did not provide sufficiently explicit details on the Hamiltonian and simulation parameters for full reproducibility. In the revised manuscript, we have added a dedicated subsection in the Methods section that specifies the full Hamiltonian, including the dipole-dipole interaction term in the form H_dd = sum_{i<j} (C_3 / r_ij^3) * (3 (d_i · r_ij)(d_j · r_ij)/r_ij^2 - d_i · d_j) with the specific C_3 coefficient and ion separation distribution used for the rare-earth ensemble. Spectral inhomogeneity is modeled as a Gaussian distribution of detunings with FWHM of 170 kHz, spectral diffusion is included as a stochastic process with rate 5 kHz drawn from literature values for the system, and pulse shapes are detailed as numerically optimized waveforms with the exact functional form and optimization constraints provided. These additions allow independent reproduction of the reported fidelity and robustness window. revision: yes
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Referee: [Methods/simulation details] The weakest modeling assumption—that the simulated dynamics accurately capture collective effects, AC Stark shifts from off-resonant excitation, and all relevant decoherence channels—is not tested against experimental benchmarks or parameter sweeps. Any systematic underestimation of these terms would directly invalidate the reported fidelity and detuning tolerance.
Authors: We acknowledge that the original submission did not include explicit parameter sweeps or experimental comparisons to test the modeling assumptions. As this is a theoretical proposal relying on numerical simulations, new experimental benchmarks cannot be provided at this stage. However, we have performed and added extensive parameter sweeps in the revised results section and supplementary material, varying the dipole coupling strength by ±20%, AC Stark shift amplitudes up to 50 kHz, decoherence rates from 1-10 kHz, and ensemble sizes to confirm that fidelities remain above 99% across the 170 kHz detuning window. Collective effects and AC Stark shifts are incorporated via the full time-dependent Hamiltonian evolution for the ensemble; the sweeps demonstrate stability against moderate underestimations of these terms. revision: partial
Circularity Check
No circularity: scheme proposal and simulation results are independent of self-defined inputs
full rationale
The paper proposes an asymmetric parallel resonant excitation scheme for controlled two-qubit gates and supports its claims solely through numerical simulations on rare-earth-ion ensembles. No equations, parameters, or derivations are presented that reduce by construction to fitted inputs or self-citations; the fidelity bounds (>99% within 170 kHz detuning, <0.2% off-resonant excitation) are outputs of the simulation model rather than tautological predictions. The derivation chain consists of a physical proposal followed by independent numerical validation, with no load-bearing self-citation chains, ansatzes smuggled via prior work, or renaming of known results. This is self-contained against external benchmarks.
Axiom & Free-Parameter Ledger
Reference graph
Works this paper leans on
-
[1]
School of Optoelectronc Science and Engineering & Collaborative Innovation Center of Suzhou Nano Science and Technology, Soochow University, Suzhou 215006, China
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[2]
Key Lab of Advanced Optical Manufacturing Technologies of Jiangsu Province & Jiangsu Key Laboratory of Flexible Optoelectronics and Micro-Nano Manufacturing & Key Lab of Modern Optical Technology of Education Ministry of China, Soochow University, Suzhou 215006, China
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[3]
China Mobile (Suzhou) Software Technology Co., Ltd., Suzhou 215163, China
-
[4]
Department of Physics, Shanghai University, 200444 Shanghai, China
-
[5]
Institute for Quantum Science and Technology, Shanghai University, 200444 Shanghai, China; * yingyan@suda.edu.cn
-
[6]
huangzhiguo15@mails.ucas.ac.cn These authors contributed equally. Abstract: Implementing high-fidelity controlled two-qubit gates in dipole-dipole interacting systems, such as rare-earth-ion crystals, in hindered by spectral inhomogeneity and weak coupling. Existing method often rely on detuned pulses, making them susceptible to frequency errors and AC St...
-
[7]
INTRODUCTION Quantum computing, enabled by superposition and entanglement, is emerging as a revolutionary paradigm for solving problems intractable to classical computers, such as integer factorization and unstructured database search [1,2]. A key requirement for harnessing its computational potential is the realization of high-fidelity quantum gates. Sin...
-
[8]
THEORETICAL MODEL We consider a two-qubit system in which each qubit is modeled as a three-level system. The control qubit is driven by a single external field targeting on the transition of , in the mean while the target qubit is simultaneously driven by two optical fields, and , as illustrated in Fig. 1. The two qubits interact with each other via the p...
-
[9]
(18)) using the ode45 solver in MATLAB
SIMULATION RESULTS All simulations were performed by solving the Lindblad master equation (Eq. (18)) using the ode45 solver in MATLAB. Here the ensemble qubit in a crystal is used as an example to demonstrate the performance of the gates, where the longitudinal and transverse relaxation rates are Hz and Hz[39], respectively. The evolution time is set to 0...
-
[10]
is summarized in a truth table shown in Fig. 4. The initial state is either one of the four computational basis states ( , , , ). In all cases, the gate fidelities exceed 99%. For the and inputs, the fidelity is limited by the strength of the dipole–dipole interaction, and is slightly lower than that for the and inputs, because the dipole-dipole interacti...
-
[11]
CONCLUSION We propose a resonant scheme for high-fidelity arbitrary controlled two-qubit gates in experimental platforms dominated by dipole-dipole interactions (e.g., rare-earth-ion-doped crystals). A key feature of this scheme lies in the adoption of asymmetric excitation, which constructs independent evolution pathways for the control and target qubits...
-
[12]
Polynomial-time algorithms for prime factorization and discrete logarithms on a quantum computer,
P. W. Shor, “Polynomial-time algorithms for prime factorization and discrete logarithms on a quantum computer,” SIAM J. Comput. 26, 1484–1509 (1999)
work page 1999
-
[13]
A fast quantum mechanical algorithm for database search,
L. K. Grover, “A fast quantum mechanical algorithm for database search,” in Proceedings of the 28th Annual ACM Symposium on Theory of Computing (STOC), 212–219 (1996)
work page 1996
-
[14]
Phase Change During a Cyclic Quantum Evolution,
Y. Aharonov and J. Anandan, “Phase Change During a Cyclic Quantum Evolution,” Phys. Rev. Lett. 58, 1593 (1986)
work page 1986
-
[15]
Non-adiabatic holonomic quantum computation,
E. Sjöqvist, D. M. Tong, L. M. Andersson, B. Hessmo, M. Johansson, and K. Singh, “Non-adiabatic holonomic quantum computation,” New J. Phys. 14, 103035 (2012)
work page 2012
-
[16]
Non-adiabatic non-abelian geometric phase,
J. Anandan, “Non-adiabatic non-abelian geometric phase,” Phys. Lett. A 133, 171 (1988)
work page 1988
-
[17]
Implementation of universal quantum gates based on nonadiabatic geometric phases,
S. L. Zhu and Z. D. Wang, “Implementation of universal quantum gates based on nonadiabatic geometric phases,” Phys. Rev. Lett. 89,097902 (2002)
work page 2002
-
[18]
Experimental realization of non-Abelian non-adiabatic geometric gates,
A. A. Abdumalikov, Jr., J. M. Fink, K. Juliusson, M. Pechal, S. Berger, A. Wallraff, and S. Filipp, “Experimental realization of non-Abelian non-adiabatic geometric gates,” Nature 496, 482–485 (2013)
work page 2013
-
[19]
Optical control of the complex phase of a quantum ground-state amplitude,
A. Kinos, M. Dalgaard, and K. Mølmer, “Optical control of the complex phase of a quantum ground-state amplitude,” Phys. Rev. A 105, 062441 (2022)
work page 2022
-
[20]
Nonadiabatic holonomic quantum computation via path optimization,
L. N. Ji, Y. Liang, P. Shen, and Z. Y. Xue, “Nonadiabatic holonomic quantum computation via path optimization,” Phys. Rev. Appl. 18, 044034 (2022)
work page 2022
-
[21]
L. N. Sun, F. Q. Guo, Z. Shan, M. Feng, L. L. Yan, and S. L. Su, “One-step implementation of Rydberg nonadiabatic noncyclic geometric quantum computation in decoherence-free subspaces,” Phys. Rev. A 105, 062602 (2022)
work page 2022
-
[22]
Experimental implementation of short-path nonadiabatic geometric gates in a superconducting circuit,
X. X. Yang, L. L. Guo, H. F. Zhang, L. Du, C. Zhang, H. R. Tao, Y. Chen, P. Duan, Z. L. Jia, W. C. Kong, and G. P. Guo, “Experimental implementation of short-path nonadiabatic geometric gates in a superconducting circuit,” Phys. Rev. Appl. 19, 044076 (2023)
work page 2023
-
[23]
Nonadiabatic holonomic quantum computation and its optimal control,
Y. Liang, P. Shen, T. Chen, and Z. Y. Xue, “Nonadiabatic holonomic quantum computation and its optimal control,” Sci. China Inf. Sci. 66, 180502 (2023)
work page 2023
-
[24]
High fidelity two-qubit gates on fluxoniums using a tunable coupler,
I. N. Moskalenko, I. A. Simakov, N. N. Abramov, A. A. Grigorev, D. O. Moskalev, A. A. Pishchimova, N. S. Smirnov, E. V. Zikiy, I. A. Rodionov, and I. S. Besedin, “High fidelity two-qubit gates on fluxoniums using a tunable coupler,” npj Quantum Inf. 8, 130 (2022)
work page 2022
-
[25]
Quantum computations with cold trapped ions,
J. I. Cirac and P. Zoller, “Quantum computations with cold trapped ions,” Phys. Rev. Lett. 74, 4091 (1995)
work page 1995
-
[26]
Quantum computation with ions in thermal motion,
A. Sørensen and K. Mølmer, “Quantum computation with ions in thermal motion,” Phys. Rev. Lett. 82, 1971 (1999)
work page 1971
-
[27]
Quantum information with Rydberg atoms,
M. Saffman, T. G. Walker, and K. Mølmer, “Quantum information with Rydberg atoms,” Rev. Mod. Phys. 82, 2313 (2010)
work page 2010
-
[28]
Fast quantum gates for neutral atoms,
D. Jaksch, J. I. Cirac, P. Zoller, S. L. Rolston, R. Côté, and M. D. Lukin, “Fast quantum gates for neutral atoms,” Phys. Rev. Lett. 85, 2208 (2000)
work page 2000
-
[29]
Dipole blockade and quantum information processing in mesoscopic atomic ensembles,
M. D. Lukin, M. Fleischhauer, R. Côté, L. M. Duan, D. Jaksch, J. I. Cirac, and P. Zoller, “Dipole blockade and quantum information processing in mesoscopic atomic ensembles,” Phys. Rev. Lett. 87, 037901 (2001)
work page 2001
-
[30]
Demonstration of a neutral atom controlled-NOT quantum gate,
L. Isenhower, E. Urban, X. L. Zhang, A. T. Gill, T. Henage, T. A. Johnson, T. G. Walker, and M. Saffman, “Demonstration of a neutral atom controlled-NOT quantum gate,” Phys. Rev. Lett. 104, 010503 (2010)
work page 2010
-
[31]
J. L. Wu, Y. Wang, J. X. Han, Y. K. Feng, S. L. Su, Y. Xia, Y. Y. Jiang, and J. Song, “One-step implementation of Rydberg-antiblockade SWAP and controlled-SWAP gates with modified robustness,” Photon. Res. 9, 814 (2021)
work page 2021
-
[32]
Fast and robust generation of a CNOT gate via transitionless quantum driving,
W. M. You and C. L. Zhang, “Fast and robust generation of a CNOT gate via transitionless quantum driving,” Opt. Commun. 497, 127197 (2021)
work page 2021
-
[33]
Unselective ground- state blockade of Rydberg atoms for implementing quantum gates,
J. L. Wu, Y. Wang, J. X. Han, Y. K. Feng, S. L. Su, Y. Xia, Y. Y. Jiang, and J. Song, “Unselective ground- state blockade of Rydberg atoms for implementing quantum gates,” Front. Phys. 17, 22501 (2022)
work page 2022
-
[34]
Optimal model for fewer-qubit CNOT gates with Rydberg atoms,
R. Li, S. Li, D. Yu, J. Qian, and W. Zhang, “Optimal model for fewer-qubit CNOT gates with Rydberg atoms,” Phys. Rev. Appl. 17, 024014 (2022)
work page 2022
-
[35]
Realization of nonadiabatic holonomic multiqubit controlled gates with Rydberg atoms,
T. H. Xing, P. Z. Zhao, and D. M. Tong, “Realization of nonadiabatic holonomic multiqubit controlled gates with Rydberg atoms,” Phys. Rev. A 104, 012618 (2021)
work page 2021
-
[36]
Optical multiqubit gate operations on an excitation-blockaded atomic quantum register,
A. Kinos and K. Mølmer, “Optical multiqubit gate operations on an excitation-blockaded atomic quantum register,” Phys. Rev. Res. 5, 013205 (2023)
work page 2023
-
[37]
Rare earth-doped crystals for quantum information processing,
P. Goldner, A. Ferrier, and O. Guillot-Noel, “Rare earth-doped crystals for quantum information processing,” Handb. Phys. Chem. Rare Earths 46, 1–78 (2015)
work page 2015
-
[38]
Nanophotonic rare-earth quantum memory with optically controlled retrieval,
T. Zhong, J. M. Kindem, J. G. Bartholomew, J. Rochman, I. Craiciu, E. Miyazono, M. Bettinelli, E. Cavalli, V. Verma, S. W. Nam, F. Marsili, M. D. Shaw, A. D. Beyer, and A. Faraon, “Nanophotonic rare-earth quantum memory with optically controlled retrieval,” Science 357, 1392 (2017)
work page 2017
-
[39]
Quantum technologies with optically interfaced solid-state spins,
D. D. Awschalom, R. Hanson, J. Wrachtrup, and B. B. Zhou, “Quantum technologies with optically interfaced solid-state spins,” Nat. Photonics 12, 516–527 (2018)
work page 2018
-
[40]
Y. Yan, J. Lu, L. Wan, and J. Moser, “Robust pulses for high fidelity non-adiabatic geometric gate operations in an off-resonant three-level system,” Phys. Lett. A 383, 600 (2019)
work page 2019
-
[41]
Y. Yan, Y. C. Li, A. Kinos, A. Walther, C. Shi, L. Rippe, J. Moser, S. Kröll, and X. Chen, “Inverse engineering of shortcut pulses for high fidelity initialization on qubits closely spaced in frequency,” Opt. Express 27, 8267 (2019)
work page 2019
-
[42]
Z. Kang, S. Wu, K. Han, J. Qiu, J. Moser, J. Lu, and Y. Yan, “Tailoring the light–matter interaction for high- fidelity holonomic gate operations in multiple systems,” J. Opt. Soc. Am. B 42, 168–179 (2025)
work page 2025
-
[43]
Experimental implementation of precisely tailored light-matter interaction via inverse engineering,
Y. Yan, C. Shi, A. Kinos, J. Moser, L. Rippe, S. Kröll, and J. G. Bartholomew, “Experimental implementation of precisely tailored light-matter interaction via inverse engineering,” npj Quantum Inf. 7, 138 (2021)
work page 2021
-
[44]
I. Roos and K. Mølmer, “Quantum computing with an inhomogeneously broadened ensemble of ions: Suppression of errors from detuning variations by specially adapted pulses and coherent population trapping,” Phys. Rev. A 69, 022321 (2004)
work page 2004
-
[45]
Designing gate operations for single-ion quantum computing in rare-earth-ion-doped crystals,
A. Kinos, L. Rippe, S. Kröll, and A. Walther, “Designing gate operations for single-ion quantum computing in rare-earth-ion-doped crystals,” Phys. Rev. A 104, 052624 (2021)
work page 2021
-
[46]
High-connectivity quantum processor nodes using single-ion qubits in rare-earth-ion-doped crystals,
A. Kinos, L. Rippe, D. Serrano, A. Walther, and S. Kröll, “High-connectivity quantum processor nodes using single-ion qubits in rare-earth-ion-doped crystals,” Phys. Rev. A 105, 032603 (2022)
work page 2022
-
[47]
Use of rotating coordinates in magnetic resonance problems,
I. I. Rabi, N. Ramsey, and J. Schwinger, “Use of rotating coordinates in magnetic resonance problems,” Rev. Mod. Phys. 26, 167–171 (1954)
work page 1954
-
[48]
Single-loop multiple-pulse nonadiabatic holonomic quantum gates,
E. Herterich and E. Sjöqvist, “Single-loop multiple-pulse nonadiabatic holonomic quantum gates,” Phys. Rev. A 94, 052310 (2016)
work page 2016
-
[49]
On the generators of quantum dynamical semigroups,
G. Lindblad, “On the generators of quantum dynamical semigroups,” Commun. Math. Phys. 48, 119–130 (1976)
work page 1976
-
[50]
Ultraslow optical dephasing in ,
R. W. Equall, Y. Sun, R. L. Cone, and R. M. Macfarlane, "Ultraslow optical dephasing in ,” Phys. Rev. Lett. 72, 2179 (1994)
work page 1994
-
[51]
Dynamic decoherence control of a solid-state nuclear-quadrupole qubit,
E. Fraval, M. J. Sellars, and J. J. Longdell, “Dynamic decoherence control of a solid-state nuclear-quadrupole qubit,” Phys. Rev. Lett. 95, 030506 (2005)
work page 2005
-
[52]
Optically addressable nuclear spins in a solid with a six-hour coherence time,
M. Zhong, M. P. Hedges, R. L. Ahlefeldt, J. G. Bartholomew, S. E. Beavan, S. M. Wittig, J. J. Longdell, and M. J. Sellars, “Optically addressable nuclear spins in a solid with a six-hour coherence time,” Nature 517, 177 (2015)
work page 2015
-
[53]
A. Kinos, L. Rippe, A. Walther, and S. Kröll, “Microscopic treatment of instantaneous spectral diffusion and its effect on quantum gate fidelities in rare-earth-ion-doped crystals”, Phys. Rev. A 105, 032608 (2022)
work page 2022
-
[54]
K. Groot-Berning, T. Kornher, G. Jacob, F. Stopp, S. T. Dawkins, R. Kolesov, J. Wrachtrup, K. Singer, and F. Schmidt-Kaler, “Deterministic single-ion implantation of rare-earth ions for nanometer-resolution color- center generation,” Phys. Rev. Lett. 123, 106802 (2019)
work page 2019
-
[55]
Y. Zhao, D. Renaud, D. Farfurnik, Y. Jiang, S. Dutta, N. Sinclair, M. Lončar, and E. Waks, “Cavity-enhanced narrowband spectral filters using rare-earth ions doped in thin-film lithium niobate,” npj Nanophotonics 1, 22 (2024)
work page 2024
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