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arxiv: cond-mat/0310516 · v1 · submitted 2003-10-22 · ❄️ cond-mat.str-el · cond-mat.mtrl-sci

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Dome-shaped magnetic phase diagram of thermoelectric layered cobaltites

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classification ❄️ cond-mat.str-el cond-mat.mtrl-sci
keywords cobaltitesmagneticdome-shapedlayerspinstatetemperatureasymptotic
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Using muon spin spectroscopy we have found that, for both Na$_x$CoO$_2$ (0.6 $\leq x \leq$ 0.9) and 3- and 4-layer cobaltites, a common low temperature magnetic state (which in some cases is manifest as an incommensurate spin density wave) forms in the CoO$_2$ planes. Here we summarize those results and report a dome-shaped relation between the transition temperature into the low-$T$ magnetic state and the composition $x$ for Na$_x$CoO$_2$ and/or the high-temperature asymptotic limit of thermopower in the more complex 3- and 4-layer cobaltites. This behavior is explained using the Hubbard model on two-dimensional triangular lattice in the CoO$_2$ plane.

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