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arxiv: cond-mat/0311161 · v1 · submitted 2003-11-07 · ❄️ cond-mat.str-el · cond-mat.mtrl-sci

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A common behavior of thermoelectric layered cobaltites: incommensurate spin density wave states in [Ca₂Co_{4/3}Cu_{2/3}O₄]_{0.62}[CoO₂] and [Ca₂CoO₃]_{0.62}[CoO₂]

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classification ❄️ cond-mat.str-el cond-mat.mtrl-sci
keywords ic-sdwspinbehaviorbelowdensityexperimentfieldincommensurate
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Magnetism of a misfit layered cobaltite [Ca$_2$Co$_{4/3}$Cu$_{2/3}$O$_4$]$_x^{\rm RS}$[CoO$_2$] ($x \sim$ 0.62, RS denotes a rocksalt-type block) was investigated by a positive muon spin rotation and relaxation ($\mu^+$SR) experiment. A transition to an incommensurate ({\sf IC}) spin density wave ({\sf SDW}) state was found below 180 K (= $T_{\rm C}^{\rm on}$); and a clear oscillation due to a static internal magnetic field was observed below 140 K (= $T_{\rm C}$). Furthermore, an anisotropic behavior of the zero-field $\mu^+$SR experiment indicated that the {\sf IC-SDW} propagates in the $a$-$b$ plane, with oscillating moments directed along the c axis. These results were quite similar to those for the related compound [Ca$_2$CoO$_3$]$_{0.62}^{\rm RS}$[CoO$_2$], {\sl i.e.}, Ca$_3$Co$_4$O$_9$. Since the {\sf IC-SDW} field in [Ca$_2$Co$_{4/3}$Cu$_{2/3}$O$_4$]$_{0.62}^{\rm RS}$[CoO$_2$] was approximately same to those in pure and doped [Ca$_2$CoO$_3$]$_{0.62}^{\rm RS}$[CoO$_2$], it was concluded that the {\sf IC-SDW} exist in the [CoO$_2$] planes.

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