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arxiv: cond-mat/0501593 · v1 · pith:4O2TFGWRnew · submitted 2005-01-25 · ❄️ cond-mat.mes-hall

Near-field Electrodynamics of Atomically Doped Carbon Nanotubes

classification ❄️ cond-mat.mes-hall
keywords waalsatomiccarbonclosecouplingdecayinteractionnanotube
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We develop a quantum theory of near-field electrodynamical properties of carbon nanotubes and investigate spontaneous decay dynamics of excited states and van der Waals attraction of the ground state of an atomic system close to a single-wall nanotube surface. Atomic spontaneous decay exhibits vacuum-field Rabi oscillations -- a principal signature of strong atom-vacuum-field coupling. The strongly coupled atomic state is nothing but a 'quasi-1D cavity polariton'. Its stability is mainly determined by the atom-nanotube van der Waals interaction. Our calculations of the ground-state atom van der Waals energy performed within a universal quantum mechanical approach valid for both weak and strong atom-field coupling demonstrate the inapplicability of conventional weak-coupling-based van der Waals interaction models in a close vicinity of the nanotube surface.

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