Direct Imaging of the First Order Spin Flop Transition in the Layered Manganite La1.4Sr1.6Mn2O7

Magnetic field induced transitions in the antiferromagnetic layered manganite La1.4Sr1.6Mn2O7 were studied using magnetization measurements and a high-resolution magneto-optical imaging technique. We report the first direct observation of the formation of ferromagnetic domains appearing at the first order spin-flop transition. The magnetization process proceeds through nucleation of polarized domains at crystal defect sites and not by domain wall motion. A small magnetic hysteresis is caused by the nucleation and annihilation of domains in the mixed state. These results establish a direct link betweeen the magnetic structure on the atomic scale as seen in neutron scattering and the macroscopic properties of the sample as seen in magnetization and conductivity measurements.