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arxiv: quant-ph/0509102 · v2 · submitted 2005-09-14 · 🪐 quant-ph

Orientation of molecules via laser-induced anti-alignment

classification 🪐 quant-ph
keywords pulseanti-alignmentmolecularorientationadditionalconsiderablydependingdifferent
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We show that field-free molecular orientation induced by a half-cycle pulse may be considerably enhanced by an additional laser pulse inducing molecular anti-alignment. Two qualitatively different enhancement mechanisms are identified depending on the pulse order, and their effects are optimized with the help of quasi-classical as well as fully quantum models.

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