Formation and relaxation of RbHe exciplexes on He nanodroplets studied by femtosecond pump and picosecond probe spectroscopy

B. Gruener; C. Giese; F. Stienkemeier; M. Mudrich; M. Weidemueller; T. Mullins

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Formation and relaxation of RbHe exciplexes on He nanodroplets studied by femtosecond pump and picosecond probe spectroscopy

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arxiv 1209.3181 v1 pith:MGNAX5BG submitted 2012-09-14 physics.atm-clus

C. Giese , T. Mullins , B. Gruener , M. Weidemueller , F. Stienkemeier , M. Mudrich This is my paper

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keywords rbheexciplexesfemtosecondformationnanodropletsproberelaxationspectra

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Vibrationally resolved photoionization spectra of RbHe exciplexes forming on He nanodroplets are recorded using femtosecond pump-probe spectroscopy with amplitude-shaped probe pulses. The time-evolution of the spectra reveals an exciplex formation time ~10ps followed by vibrational relaxation extending up to >1ns. This points to an indirect, time-delayed desorption process of RbHe off the He surface.

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