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Unexpected Universality in the Viscosity of Metallic Liquids

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arxiv 1407.7558 v1 pith:URXQPKXH submitted 2014-07-28 cond-mat.soft cond-mat.dis-nn

classification cond-mat.softcond-mat.dis-nn
keywords temperatureviscosityextrapolatedglassinfiniteliquidsmetallictransition
verification ladder T0 review T1 audit T2 compute T3 formal
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The range of the magnitude of the liquid viscosity as a function of the temperature (T) is one of the most impressive of any physical property, changing by approximately 17 orders of magnitude from its extrapolated value at infinite temperature to that at the glass transition. We present experimental measurements of containerlessly processed metallic liquids that reveal that the ratio of the viscosity to its extrapolated infinite temperature value follows a universal function of Tcoop/T. The temperature Tcoop corresponds to the onset of cooperative motion and is strongly correlated with the glass transition temperature. On average the extrapolated infinite temperature viscosity is found to be nh, where h is Planck's constant and n is the particle number density. A surprising universality in the viscosity of metallic liquids and its relation to the glass transition is demonstrated.

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