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Magnetic ordering in the ultra-pure site-diluted spin chain materials SrCu_(1-x)Ni_xO₂

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arxiv 1603.04090 v2 pith:XXSEMFFT submitted 2016-03-13 cond-mat.str-el

Magnetic ordering in the ultra-pure site-diluted spin chain materials SrCu$_{1-x}$Ni$_x$O$_2$

classification cond-mat.str-el
keywords magneticorderingspinamountchainprevioussrcuultra-pure
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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abstract

Muon spin rotation technique is used to study magnetic ordering in ultra-pure samples of SrCu$_{1-x}$Ni$_x$O$_2$, an archetypical $S=1/2$ antiferromagnetic Heisenberg chain system with a small amount of $S=1$ defects. The ordered state in the parent compound is shown to be highly homogeneous, contrary to previous report [M. Matsuda et al., Phys. Rev. B \textbf{55}, R11953 (1997)]. Even minute amount of Ni impurities result in inhomogeneous order and a decrease of the transition temperature. At as little as $0.5$~\% Ni concentration, magnetic ordering is entirely suppressed. The results are compared to previous theoretical studies of weakly coupled spin chains with site-defects.

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