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Revealing the Atomic Site-Dependent g Factor within a Single Magnetic Molecule via the Extended Kondo Effect

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arxiv 2004.02741 v1 pith:37WXEAJL submitted 2020-04-06 cond-mat.mes-hall

Liwei Liu , Kai Yang , Yuhang Jiang , Boqun Song , Wende Xiao , Shiru Song , Shixuan Du , Min Ouyang
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Werner A. Hofer Antonio H. Castro Neto Hong-Jun Gao
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classification cond-mat.mes-hall
keywords moleculesinglefactoratomiceffectextendedkondomagnetic
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The site-dependent g factor of a single magnetic molecule, with intramolecular resolution, is demonstrated for the first time by low-temperature, high-magnetic-field scanning tunneling microscopy of dehydrogenated Mn-phthalocyanine molecules on Au(111). This is achieved by exploring the magneticfield dependence of the extended Kondo effect at different atomic sites of the molecule. Importantly, an inhomogeneous distribution of the g factor inside a single molecule is revealed. Our results open up a new route to access local spin properties within a single molecule.

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