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Finite-temperature magnetic properties of Sm2Fe17Nx using an ab-initio effective spin model

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arxiv 2012.08120 v3 pith:KQ53V4CW submitted 2020-12-15 cond-mat.mtrl-sci

Shogo Yamashita , Daiki Suzuki , Takuya Yoshioka , Hiroki Tsuchiura , Pavel Novák This is my paper · ORCID
classification cond-mat.mtrl-sci
keywords modelmagneticpropertiesconfigurationcurveseffectivefinite-temperaturemagnetization
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In this study, we investigate the finite-temperature magnetic properties of Sm2Fe17Nx (x = 0,3) using an effective spin model constructed based on the information obtained by first-principles calculations. We find that assuming the plausible trivalent Sm3+ configuration results in a model that can satisfactorily describe the magnetization curves of Sm2Fe17N3. By contrast, the model based on the divalent Sm2+ configuration is suitable to reproduce the magnetization curves of Sm2Fe17. These results expand the understanding of how electronic structure affects the magnetic properties of these compounds.

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