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Single molecule superradiance for optical cycling
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Single molecule superradiance for optical cycling
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Herein, we show that single molecules containing multiple optical cycling centers (CaO moieties) can exhibit superradiant phenomena. We demonstrate the accuracy of the Frenkel exciton model at describing these superradiant states via comparisons to high-level electronic structure methods. We then rationally design molecules with superradiant properties optimized for laser cooling. Lastly, we demonstrate how multi-photon superradiant phenomena can occur in these novel molecular systems.
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Cited by 1 Pith paper
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Molecular Quantum Control Algorithm Design by Reinforcement Learning
Reinforcement learning designs quantum-logic pulse sequences to prepare H3O+ (130 states) and CaH+ molecular ions in pure states from thermal populations.
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