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Spinons in a new Shastry-Sutherland lattice magnet Pr$_2$Ga$_2$BeO$_7$
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abstract
Identifying the elusive spinon excitations in quantum spin liquid (QSL) materials is what scientists have long sought for. Recently, thermal conductivity ($\kappa$) has emerged to be a decisive probe because the fermionic nature of spinons leads to a characteristic nonzero linear $\kappa_0/T$ term while approaching zero Kelvin. So far, only a few systems have been reported to exhibit such term. Here, we report a $\kappa_0/T \approx$ 0.01 WK$^{-2}$m$^{-1}$, the largest $\kappa_0/T$ value ever observed in magnetic oxide QSL candidates, in a new quantum magnet Pr$_2$Ga$_2$BeO$_7$ with a Shastry-Sutherland lattice (SSL). Its QSL nature is further supported by the power-law temperature dependence of the specific heat, a plateau of muon spin relaxation rate, and gapless inelastic neutron spectra. Our theoretical analysis reveals that the introduction of XY spin anisotropy is the key for Pr$_2$Ga$_2$BeO$_7$ to be the first QSL realized on the SSL, after more than four decades of extensive studies on this celebrated magnetically frustrated lattice.
Forward citations
Cited by 2 Pith papers
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Spiral Phase and Phase Diagram of the $S$=1/2 XXZ Model on the Shastry-Sutherland Lattice
A new incommensurate spiral phase is found in the S=1/2 XXZ Shastry-Sutherland model at small anisotropy, while the empty-plaquette phase narrows as anisotropy grows.
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Quantum entanglement of XY-type spin dimers in Shastry-Sutherland lattice
BaCe2ZnS5 is a quantum paramagnet whose intra-dimer exchange is XY-type, giving an entangled ground state (|↑↑> - |↓↓>)/√2 instead of a Heisenberg singlet.
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