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Interplay between electronic and lattice superstructures in La$_{2-x}$Ca$_{x}$CuO$_{4}$
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abstract
Complex oxides are well known to develop oxygen ordering patterns with well defined periodicities, but their interplay with electronic correlations remains largely unexplored. Here, we report resonant and non-resonant x-ray diffraction data indicating a four-unit-cell periodic superstructure related to oxygen vacancy ordering in La$_{2-x}$Ca$_{x}$CuO$_{4}$ films with doping levels from the underdoped ($x = 0.15$) to the extremely overdoped ($x = 0.50$) regime. Whereas the lattice superstructure is temperature independent up to 300 K, a strongly temperature dependent electronic charge density wave (CDW) is observed in the underdoped and slightly overdoped regimes ($x\leq0.20$). The periodicity, in-plane and out-of-plane correlation lengths of the CDW are locked in by the lattice superstructure. Our results highlight the necessity to consider lattice and electronic energetics on equal footing in the high-temperature oxygen-disordered phase to explain oxygen ordering phenomena in complex oxides.
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Cited by 1 Pith paper
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Evolution of spin excitations in superconducting La$_{2-x}$Ca$_{x}$CuO$_{4-\delta}$ from the underdoped to the heavily overdoped regime
RIXS shows that high-energy paramagnons in LCCO cuprate films persist to x=0.50 and are insensitive to the extended superconducting dome, indicating they are not the primary pairing glue.
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