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Cascade of strongly correlated quantum states in a partially filled kagome flat band

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arxiv 2409.06933 v1 pith:4I2OR2GP submitted 2024-09-11 cond-mat.str-el cond-mat.mes-hall

classification cond-mat.str-elcond-mat.mes-hall
keywords flatstatebandstatescorrelatedcoulombdopingelectronic
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abstract

Coulomb interactions among charge carriers that occupy an electronic flat band have a profound impact on the macroscopic properties of materials. At sufficient strength, these interactions can give rise to captivating phenomena such as quantum criticality, Mott-Hubbard states, and unconventional superconductivity. The appearance of these characteristics sensitively depends on the number of electrons occupying the flat band states. In this work, we present experimental evidence obtained from scanning tunneling microscopy measurements for a cascade of strongly correlated states appearing in the partially occupied kagome flat bands of Co$_{1-x}$Fe$_x$Sn whose filling can be controlled by the Fe-doping level $x$. At elevated temperatures ($T\geq16\,K$), we detect a nematic electronic state across a broad doping range $0.05<x<0.25$. The comparison with model calculations reveals that strong Coulomb interactions ($U>100\,$meV) blend the states of two $3d$-orbital derived flat bands and impart a nematic order parameter. This state serves as the parent phase of a strongly correlated phase diagram: At lower temperatures $T<16\,$K, we find spectroscopic evidence for an orbital-selective Mott state enabled by the $3d$-orbital degeneracy of the Co atom. This state can only be detected in samples with ideal Fe doping ($x=0.17$) and descends into pseudogap phases upon electron and hole doping. At $T<8\,$K, the pseudogap phase evolves into another nematic low temperature state. Our observations demonstrate that the electronic ground state of a kagome flat band depends on the complex interplay between strong Coulomb repulsion, $3d$-orbital degeneracy, and flat band filling fraction at different temperatures.

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  1. Room temperature observation of the anomalous in-plane Hall effect in epitaxial thin films of a Weyl ferromagnet

    cond-mat.mes-hall 2025-01 conditional novelty 6.0 of 10

    A temperature-independent anomalous in-plane Hall conductivity of about 0.8 S/cm is observed between 100 and 300 K in spin-canted epitaxial Fe3Sn films and attributed to Weyl-point Berry curvature.

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