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Theory of potential impurity scattering in pressurized superconducting La$_3$Ni$_2$O$_7$

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arxiv 2411.01935 v1 pith:3ZPRFNY7 submitted 2024-11-04 cond-mat.supr-con cond-mat.str-el

classification cond-mat.supr-concond-mat.str-el
keywords wavesuperconductingla-327statebehaviorimpuritysymmetryconcentration
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abstract

Recently discovered high-T$_c$ superconductivity in pressurized bilayer nickelate La$_3$Ni$_2$O$_7$ (La-327) is believed to be driven by the non-phononic repulsive interaction. Depending on the strength of the interlayer repulsion, the symmetry of the superconducting order parameter is expected to be either $d$-wave or sign-changing bonding-antibonding $s_{\pm}$-wave. Unfortunately, due to the need of high pressure to reach superconducting phase, conventional spectroscopic probes to validate the symmetry of the order parameter are hard to use. Here, we study the effect of the point-like non-magnetic impurities on the superconducting state of La-327 and show that $s_{\pm}$-wave and $d$-wave symmetries show a very different behavior as a function of impurity concentration, which can be studied experimentally by irradiating the La-327 samples by electrons prior applying the pressure. While $d-$wave superconducting state will be conventionally suppressed, the $s_{\pm}$-wave state shows more subtle behavior, depending on the asymmetry between bonding and antibonding subspaces. For the electronic structure, predicted to realize in La-327, the $s_{\pm}-$wave state will be robust against complete suppression and the transition temperature, $T_c$ demonstrates a transition from convex to concave behavior, indicating a crossover from $s_{\pm}$-wave to $s_{++}$-wave symmetry as a function of impurity concentration. We further analyze the sensitivity of the obtained results with respect to the potential electronic structure modification.

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Cited by 2 Pith papers

Reviewed papers in the Pith corpus that reference this work. Sorted by Pith novelty score. Full citation record

  1. Orbital-selective electron correlations in high-$T_{\rm c}$ bilayer nickelates: from a global phase diagram to implications for spectroscopy

    cond-mat.supr-con 2024-12 conditional novelty 7.0 of 10

    A bilayer two-orbital Hubbard model of La3Ni2O7 shows orbital-selective correlations, with z2 electrons forming interlayer singlets, that reproduce key ARPES and optical conductivity features.

  2. Magnetic Order in bilayer Ruddlesden-Popper Nickelates

    cond-mat.supr-con 2026-07 conditional novelty 6.0 of 10

    Combining superexchange with RKKY interactions between orbital-selective local moments reproduces the (π/2,π/2) magnetic order and ~80 meV spin excitations of bilayer nickelate La₃Ni₂O₇.

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