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U(1) Dirac quantum spin liquid candidate in triangular-lattice antiferromagnet CeMgAl$_{11}$O$_{19}$

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arxiv 2502.19259 v1 pith:CQSHPPUR submitted 2025-02-26 cond-mat.str-el

classification cond-mat.str-el
keywords spinliquidquantumdependencemagneticstatesusceptibilitytemperature
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abstract

Quantum spin liquid represents an intriguing state where electron spins are highly entangled yet spin fluctuation persists even at 0 K. Recently, the hexaaluminates \textit{R}MgAl$_{11}$O$_{19}$ (\textit{R} = rare earth) have been proposed to be a platform for realizing the quantum spin liquid state with dominant Ising anisotropic correlations. Here, we report detailed low-temperature magnetic susceptibility, muon spin relaxation, and thermodynamic studies on the CeMgAl$_{11}$O$_{19}$ single crystal. Ising anisotropy is revealed by magnetic susceptibility measurements. Muon spin relaxation and ac susceptibility measurements rule out any long-range magnetic ordering or spin freezing down to 50 mK despite the onset of spin correlations below $\sim$0.8 K. Instead, the spins keep fluctuating at a rate of 1.0(2) MHz at 50 mK. Specific heat results indicate a gapless excitation with a power-law dependence on temperature, $C_m(T) \propto T^{\alpha}$. The quasi-quadratic temperature dependence with $\alpha$ = 2.28(4) in zero field and linear temperature dependence in 0.25 T support the possible realization of the U(1) Dirac quantum spin liquid state.

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  1. Quantum disordered ground state and relative proximity to an exactly solvable model in the frustrated magnet CeMgAl$_{11}$O$_{19}$

    cond-mat.str-el 2025-06 conditional novelty 6.0 of 10

    Magnetization and heat-capacity data place CeMgAl11O19 at Jz/J⊥ ≈ -0.22, farther from the solvable quantum-critical point than the previously reported -0.43, and point to structural disorder as the driver of its quant...

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