Sub-5-fs compression and synchronization of relativistic electron bunches enabled by a high-gradient α-magnet and low-jitter photoinjector

Generating high-brightness relativistic electron bunches with few-femtosecond duration, while simultaneously achieving few-fs synchronization with ultrafast lasers, remains an outstanding challenge at the frontier of accelerator physics and ultrafast science. In this Letter, we present the beam physics and experimental demonstration of a new method that, for the first time, enables simultaneous control of bunch duration and synchronization with few-fs precision. Timing stabilization is achieved using a tailored high-gradient $\alpha$-magnet that optimizes the correlation between time of flight and momentum, together with a photocathode RF gun designed to suppress the effect of RF-to-laser timing jitter. Compression is realized by manipulating the time-momentum correlation in phase space, primarily through space-charge effects. Sub-5-fs rms bunch duration and synchronization are demonstrated. This method establishes a new regime in electron bunch control, unlocking new capabilities for ultrafast beam physics and applications.