arxiv: 1401.3265 · v1 · pith:7QCOYHVUnew · submitted 2014-01-14 · ❄️ cond-mat.str-el · cond-mat.mtrl-sci

Evidence for SrHo2O4 and SrDy2O4 as model J1-J2 zig-zag chain materials

Amy Poole , Vladimir Pomjakushin , Anne-Christine Uldry , Bernhard Delley , Bobby Prevost , Alexandre Desilets-Benoit , Andrea D Bianchi , Robert I Bewley

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Britt R Hansen Thomasz Klimczuk Robert J Cava Michel Kenzelmann

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classification ❄️ cond-mat.str-el cond-mat.mtrl-sci

keywords chaincorrelationsdiffractioninteractionsmaterialsmeasurementssrdy2o4srho2o4

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Neutron diffraction and inelastic spectroscopy is used to characterize the magnetic Hamiltonian of SrHo2O4 and SrDy2O4. Through a detailed computation of the crystal-field levels we find site- dependent anisotropic single-ion magnetism in both materials and diffraction measurements show the presence of strong one-dimensional spin correlations. Our measurements indicate that competing interactions of the zig-zag chain, combined with frustrated interchain interactions, play a crucial role in stabilizing spin-liquid type correlations in this series.

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Evidence for SrHo2O4 and SrDy2O4 as model J1-J2 zig-zag chain materials

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