Harmonic entanglement with second-order non-linearity

We investigate the second-order non-linear interaction as a means to generate entanglement between fields of differing wavelengths. And show that perfect entanglement can, in principle, be produced between the fundamental and second harmonic fields in these processes. Neither pure second harmonic generation, nor parametric oscillation optimally produce entanglement, such optimal entanglement is rather produced by an intermediate process. An experimental demonstration of these predictions should be imminently feasible.