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arxiv: 1101.5457 · v1 · pith:BVICZ5OTnew · submitted 2011-01-28 · ❄️ cond-mat.str-el · cond-mat.supr-con

Sr3Co2O6: a possible frustrated spin-chain material

X. X. Wang , J. J. Li , Y. G. Shi , Y. Tsujimoto , Y. F. Guo , S. B. Zhang , Y. Matsushita , M. Tanaka
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Y. Katsuya K. Kobayashi K. Yamaura E. Takayama-Muromachi
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classification ❄️ cond-mat.str-el cond-mat.supr-con
keywords sr3co2o6structurek4cdcl6-typemagneticperovskitespin-chainambientanalogue
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A dense phase of a post-layered perovskite Sr3Co2O6 was created by a high-pressure and high-temperature synthetic route and quenched to ambient conditions. The structure of Sr3Co2O6 was determined by synchrotron X-ray powder diffraction. Sr3Co2O6 crystallizes in the K4CdCl6-type structure (an infinite chain-type structure), which is 6% denser than the known, iso-compositional layered perovskite Sr3Co2O7-d (d~1). The K4CdCl6-type Sr3Co2O6 shows complex magnetic behavior reflecting the spin-chain nature as well as the analogue oxides Ca3Co2O6 and Ca3CoRhO6, whose microscopic magnetic origin is still highly debated.

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