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Electronic instability, layer selectivity and Fermi arcs in La$_3$Ni$_2$O$_7$

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arxiv 2403.12831 v3 pith:CGPAXD5P submitted 2024-03-19 cond-mat.str-el cond-mat.supr-con

classification cond-mat.str-elcond-mat.supr-con
keywords electronicarcslayerselectivitystructurecorrelatedfermiflat-band
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abstract

Using advanced dynamical mean-field theory on a realistic level we study the normal-state correlated electronic structure of the high-pressure superconductor La$_3$Ni$_2$O$_7$ and compare the features of the conventional bilayer (2222) Ruddelsden-Popper crystal structure with those of a newly-identified monolayer-trilayer (1313) alternation. Both structural cases display Ni-$d_{z^2}$ flat-band character at low-energy, which drives an electronic instability with a wave vector ${\bf q_{\rm I}}=(0.25,0.25,q_z)$ at ambient pressure, in line with recent experimental findings. The 1313 electronic structure exhibits significant layer selectivity, rendering especially the monolayer part to be Mott-critical. At high pressure, this layer selectivity weakens and the 1313 fermiology displays arcs reminiscent to those of high-$T_c$ cuprates. In contrast to dominant inter-site self-energy effects in the latter systems, here the Fermi arcs are the result of the multiorbital and multilayer interplay within a correlated flat-band scenario.

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  1. Signature of superconductivity in pressurized La4Ni3O10-x single crystals grown at ambient pressure

    cond-mat.supr-con 2025-01 conditional novelty 5.0 of 10

    Ambient-pressure flux-grown La4Ni3O10-x single crystals show a pressure-induced resistance drop and magnetic-field-suppressed Tc near 30 K at 77.9 GPa, a superconductivity signature matching floating-zone crystals.

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