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arxiv: 0704.1017 · v2 · pith:COCSP2ELnew · submitted 2007-04-08 · ❄️ cond-mat.str-el · cond-mat.stat-mech

Magnetic susceptibility and specific heat of the spin-1/2 Heisenberg model on the kagome lattice and experimental data on ZnCu3(OH)6Cl2

classification ❄️ cond-mat.str-el cond-mat.stat-mech
keywords experimentalheatheisenbergkagomemodelspecificsusceptibilityzncu3
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We compute the magnetic susceptibility and specific heat of the spin-1/2 Heisenberg model on the kagome lattice with high-temperature expansions and exact diagonalizations. We compare the results with the experimental data on ZnCu3(OH)6Cl2 obtained by Helton et al. [Phys. Rev. Lett. 98, 107204 (2007)]. Down to k_BT/J~0.2, our calculations reproduce accurately the experimental susceptibility, with an exchange interaction J~190K and a contribution of 3.7% of weakly interacting impurity spins. The comparison between our calculations of the specific heat and the experiments indicate that the low-temperature entropy (below ~20K) is smaller in ZnCu3(OH)6Cl2 than in the kagome Heisenberg model, a likely signature of other interactions in the system.

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