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Plasmon-enhanced second harmonic generation in semiconductor quantum dots close to metal nanoparticles

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arxiv 1106.2253 v2 pith:DQLEQ67Q submitted 2011-06-11 cond-mat.mes-hall

classification cond-mat.mes-hall
keywords enhancementsilverclosedotsharmonicnanoparticlesomegaquantum
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abstract

We report the enhancement of the optical second harmonic signal in non-centrosymmetric semiconductor CdS quantum dots, when they are placed in close contact with isolated silver nanoparticles. The intensity enhancement is about 1000. We also show that the enhancement increases when the incoming laser frequency $\omega$ is tuned toward the spectral position of the silver plasmon at $2\omega$, proving that the silver nanoparticle modifies the nonlinear emission.

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