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Site Selectivity on Chalcogen Atoms in Superconducting La(O,F)BiSSe

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arxiv 1412.8387 v2 pith:EML5WUM3 submitted 2014-12-29 cond-mat.supr-con

Masashi Tanaka , Takuma Yamaki , Yoshitaka Matsushita , Masaya Fujioka , Saleem J. Denholme , Takahide Yamaguchi , Hiroyuki Takeya , Yoshihiko Takano This is my paper · ORCID
classification cond-mat.supr-con
keywords superconductingsingleatomsbissecrystalcrystalsmagneticsite
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abstract

Single crystals of La(O,F)BiSSe were successfully grown by a CsCl flux method. Single crystal X-ray structural analysis revealed that the crystal structure is isostructural with BiS$_2$- or BiSe$_2$-based compounds with space group $P4/nmm$ (lattice parameters $a$ = 4.1110(2) {\AA}, $c$ = 13.6010(7) {\AA}). However, the S atoms are selectively occupied at the apical site of the Bi-SSe pyramids in the superconducting layer. The single crystals show a superconducting transition at 4.2 K in the magnetic susceptibility and resistivity measurement. The superconducting anisotropic parameter is determined to be 34 from its upper critical magnetic field. The anisotropy is in the same range with that of other members of the La(O,F)BiCh$_2$ ($Ch$ = S, Se) family under ambient pressure.

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