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Magnetic field-induced phases and spin Hamiltonian in Cs2CoBr4

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arxiv 2311.10535 v2 pith:GGRTRZPF submitted 2023-11-17 cond-mat.str-el

Magnetic field-induced phases and spin Hamiltonian in Cs2CoBr4

classification cond-mat.str-el
keywords magneticspincs2cobr4hamiltonianneutronabsorptionacrossadditional
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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Magnetic structures and spin excitations are studied across the phase diagram of the geometrically frustrated S = 3/2 quantum antiferromagnet Cs2CoBr4 in magnetic fields applied along the magnetic easy axis, using neutron diffraction, inelastic neutron scattering and THz absorption spectroscopy. The data are analyzed, where appropriate, using extended SU (4) linear spin wave theory. A minimal magnetic Hamiltonian is proposed based on measurements in the high field polarized state. It deviates considerably from the previously considered models. Additional dilatometry experiments highlight the importance of magnetoelastic coupling in this system.

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