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Electronic band structure of BaCo$_{2}$As$_2$: a fully-doped ferropnictide with reduced electronic correlations

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arxiv 1210.5576 v1 pith:H3RLD5I5 submitted 2012-10-20 cond-mat.str-el cond-mat.supr-con

classification cond-mat.str-elcond-mat.supr-con
keywords electronicbacobandstructurecorrelationsfermisurfaceagreement
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abstract

We report an angle-resolved photoemission spectroscopy investigation of the Fermi surface and electronic band structure of BaCo$_{2}$As$_2$. Although its quasi-nesting-free Fermi surface differs drastically from that of its Fe-pnictide cousins, we show that the BaCo$_{2}$As$_2$ system can be used as an approximation to the bare unoccupied band structure of the related BaFe$_{2-x}$Co$_x$As$_2$ and Ba$_{1-x}$K$_x$Fe$_2$As$_2$ compounds. However, our experimental results, in agreement with dynamical mean field theory calculations, indicate that electronic correlations are much less important in BaCo$_{2}$As$_2$ than in the ferropnictides. Our findings suggest that this effect is due to the increased filling of the electronic 3$d$ shell in the presence of significant Hund's exchange coupling.

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