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arxiv: cond-mat/0410065 · v2 · pith:KL62II6Knew · submitted 2004-10-04 · ❄️ cond-mat.mtrl-sci · cond-mat.str-el

Inhomogeneous level splitting in Pr_(2-x)Bi_xRu₂O₇

classification ❄️ cond-mat.mtrl-sci cond-mat.str-el
keywords approxhbaromegaaccountantiferromagneticbroadcontinuousdata
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We report that Bi doping drives Pr$_x$Bi$_{2-x}$Ru$_2$O$_7$ from an antiferromagnetic insulator ($x=2$) to a metallic paramagnet ($x\approx 1$) with a broad low $T$ maximum in $C/T$. Neutron scattering reveals local low energy spin excitations ($\hbar\omega\approx 1$ meV) with a spectrum that is unaffected by heating to $k_BT>>\hbar\omega$. We show that a continuous distribution of splittings of the non-Kramers Pr$^{3+}$ ground state doublet such as might result from various types of lattice strain can account for all the data.

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