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Resonance Anomalous Surface X-ray Scattering

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arxiv cond-mat/0510235 v1 pith:LMMCA5KR submitted 2005-10-10 cond-mat.mtrl-sci

Andreas Menzel , Kee-Chul Chang , Vladimir Komanicky , Hoydoo You , Yong S. Chu , Yuriy V. Tolmachev , John J. Rehr This is my paper · ORCID
classification cond-mat.mtrl-sci
keywords polarizationrasxssurfacedependencescatteringadsorptionanodicanomalous
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Resonance anomalous surface x-ray scattering (RASXS) technique was applied to electrochemical interface studies. It was used to determine the chemical states of electrochemically formed anodic oxide monolayers on platinum surface. It is shown that RASXS exhibits strong polarization dependence when the surface is significantly modified. The polarization dependence is demonstrated for three examples; anodic oxide formation, sulfate adsorption, and CO adsorption on platinum surfaces. s- and p- polarization RASXS data were simulated with the latest version of ab initio multiple scattering calculations (FEFF8.2). Elementary theoretical considerations are also presented for the origin of the polarization dependence in RASXS.

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