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Experimentally tunable QED in dipolar-octupolar quantum spin ice

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arxiv 2312.11641 v2 pith:QEOKDVNC submitted 2023-12-18 cond-mat.str-el

Experimentally tunable QED in dipolar-octupolar quantum spin ice

classification cond-mat.str-el
keywords emergentquantumdo-qsiexperimentallyfieldspindipolar-octupolareqed
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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We propose a readily achievable experimental setting where an external magnetic field is used to tune the emergent quantum electrodynamics (eQED) of dipolar-octupolar quantum spin ice (DO-QSI). In $U(1)_\pi$ DO-QSI -- the proposed ground state of QSI candidates Ce$_2$Zr$_2$O$_7$, Ce$_2$Sn$_2$O$_7$ and Ce$_2$Hf$_2$O$_7$ -- we show that the field can be used to control the emergent speed of light (and, consequently, the emergent fine structure constant). Depending on the field's alignment with the crystal, one may induce different speeds for the two polarizations of the emergent photons, in a fascinating analogue of the electro-optic Kerr effect. In $U(1)_0$ DO-QSI -- yet to be uncovered experimentally -- we find a number of unusual field-induced transitions, including a transition between $0$- and $\pi$-flux QSI phases, as well as phases with frustrated flux configurations. We discuss experimental signatures of these effects in the spinon excitation spectrum, which can be readily accessed for instance in inelastic neutron scattering measurements. Our proposal opens the gate to a plethora of experimentally accessible, engineerable eQED phenomena in the emergent universes of quantum spin ice.

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Cited by 3 Pith papers

Reviewed papers in the Pith corpus that reference this work. Sorted by Pith novelty score.

  1. $q$-state Potts ice

    cond-mat.str-el 2026-01 conditional novelty 7.0

    Potts ice models map onto su(Nc) gauge theory, with root-charge excitations, unique flavor-changing interactions for Nc>2, and a conjectured flux-liquid vacuum.

  2. Spectroscopic Demarcation of Emergent Photons and Spinons in a Dipolar-Octupolar Quantum Spin Liquid

    cond-mat.str-el 2026-01 conditional novelty 6.0

    A weak [111] magnetic field suppresses the emergent-photon weight but leaves the spinon continuum intact in Ce2Zr2O7, giving a new field-tuning protocol to demarcate fractionalized excitations.

  3. Magnetization and magnetostriction measurements of the dipole-octupole quantum spin ice candidate Ce2Hf2O7

    cond-mat.str-el 2025-09 conditional novelty 6.0

    Magnetization and magnetostriction data on Ce2Hf2O7 show a kink anomaly best reproduced by a Hamiltonian with dominant octupole interactions, supporting an octupole-based quantum spin ice ground state.