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EUV ionization of pure He nanodroplets: Mass-correlated photoelectron imaging, Penning ionization and electron energy-loss spectra

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arxiv 1305.3726 v1 pith:QV32QJKM submitted 2013-05-16 physics.atm-clus

D. Buchta , S. R. Krishnan , N. B. Brauer , M. Drabbels , P. O'Keeffe , M. Devetta , M. Di Fraia , C. Callegari
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R. Richter M. Coreno K. C. Prince F. Stienkemeier R. Moshammer M. Mudrich
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classification physics.atm-clus
keywords ionizationdropletscoincidenceimagingnanodropletsphotoelectronpurespectra
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The ionization dynamics of pure He nanodroplets irradiated by EUV radiation is studied using Velocity-Map Imaging PhotoElectron-PhotoIon COincidence (VMI-PEPICO) spectroscopy. We present photoelectron energy spectra and angular distributions measured in coincidence with the most abundant ions He+, He2+, and He3+. Surprisingly, below the autoionization threshold of He droplets we find indications for multiple excitation and subsequent ionization of the droplets by a Penning-like process. At high photon energies we evidence inelastic collisions of photoelectrons with the surrounding He atoms in the droplets.

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