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Static linear density response from X-ray Thomson scattering measurements: a case study of warm dense beryllium

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arxiv 2504.13611 v2 pith:SHFVGF5F submitted 2025-04-18 physics.plasm-ph physics.chem-ph

classification physics.plasm-phphysics.chem-ph
keywords densitydenseemphlinearresponsewarmberylliumestimate
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abstract

Linear response theory is ubiquitous throughout physics and plays a central role in the theoretical description of warm dense matter -- an extreme state that occurs within compact astrophysical objects and that is traversed on the compression path of a fuel capsule in inertial confinement fusion applications. Here we show how one can relate the static linear density response function to X-ray Thomson scattering (XRTS) measurements, which opens up new possibilities for the diagnostics of extreme states of matter, and for the rigorous assessment and verification of theoretical models and approximations. As a practical example, we consider an XRTS data set of warm dense beryllium taken at the National Ignition Facility [T.~D\"oppner \emph{et al.}, \textit{Nature} \textbf{618}, 270-275 (2023)]. The comparison with state-of-the-art \emph{ab initio} path integral Monte Carlo (PIMC) simulations [T.~Dornheim \emph{et al.}, \textit{Nature Commun.}~(in print), arXiv:2402.19113] gives us a best estimate of the mass density of $\rho=18\pm6\,$g/cc, which is consistent with previous PIMC and density functional theory based studies, but rules out the original estimate of $\rho=34\pm4\,$g/cc based on a Chihara model fit.

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Cited by 3 Pith papers

Reviewed papers in the Pith corpus that reference this work. Sorted by Pith novelty score. Full citation record

  1. Reconciling chemical models of X-ray Thomson Scattering with the Bethe $f$-sum rule

    physics.plasm-ph 2026-07 conditional novelty 6.0 of 10

    Including bound-bound transitions and exact Coulomb bound-free matrix elements makes the Chihara model satisfy the Bethe f-sum rule for hydrogen-like atoms.

  2. Dielectric formalism of the 2D uniform electron gas at finite temperatures

    cond-mat.str-el 2026-01 conditional novelty 6.0 of 10

    Finite-temperature 2D electron gas: STLS and HNC dielectric theories are benchmarked against new path-integral Monte Carlo data, with a fit of the exchange-correlation free energy.

  3. Exact series expansion for even frequency moments of the dynamic structure factor

    physics.plasm-ph 2025-06 conditional novelty 6.0 of 10

    Even frequency moments of S(q,ω) are expanded in a Bernoulli series over odd moments, and the truncated sums give useful estimates of the second, fourth and fifth moments for weakly degenerate electron gases.

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