Dynamical exchange and phase induced switching of a localized molecular spin
classification
❄️ cond-mat.mes-hall
keywords
spinlocalizedswitchingdynamicaldynamicsexchangefieldsmolecular
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The dynamics of a localized molecular spin under the influence of external voltage pulses is addressed using a generalized spin equation of motion. The approach incorporates anisotropic fields, non-equilibrium conditions, and non-adiabatic dynamics. By application of a voltage pulse of temporal length $\tau$, a recurring $4\pi$-periodic switching of the localized spin is observed. The switching phenomena can be explained by dynamical exchange interactions, internal transient fields, and self-interactions acting on the localized spin moment.
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