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An intense, cold, velocity-controlled molecular beam by frequency-chirped laser slowing

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arxiv 1605.06055 v2 pith:TO5EEWVH submitted 2016-05-19 physics.atom-ph

classification physics.atom-ph
keywords slowingbeamfrequency-chirpedvelocitylasermethodmolecularcold
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abstract

Using frequency-chirped radiation pressure slowing, we precisely control the velocity of a pulsed CaF molecular beam down to a few m/s, compressing its velocity spread by a factor of 10 while retaining high intensity: at a velocity of 15~m/s the flux, measured 1.3~m from the source, is 7$\times$10$^{5}$ molecules per cm$^{2}$ per shot in a single rovibrational state. The beam is suitable for loading a magneto-optical trap or, when combined with transverse laser cooling, improving the precision of spectroscopic measurements that test fundamental physics. We compare the frequency-chirped slowing method with the more commonly used frequency-broadened slowing method.

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Cited by 1 Pith paper

Reviewed papers in the Pith corpus that reference this work. Sorted by Pith novelty score. Full citation record

  1. Controlling rovibrational state populations of polar molecules in inhomogeneous electric fields of the Stark deceleration: molecular dynamics and quantum chemistry simulations

    physics.atom-ph 2025-06 conditional novelty 6.0 of 10

    A modified SCRAP technique using the decelerator's time-varying dc electric field as the chirp can achieve >99.5% population inversion between weak-field- and strong-field-seeking states of ammonia, improving Stark de...

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