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arxiv 2101.10045 v2 pith:TZNTCY6H submitted 2021-01-25 cond-mat.str-el

In-situ electric field control of THz non-reciprocal directional dichroism in the multiferroic Ba₂CoGe₂O₇

classification cond-mat.str-el
keywords electricnon-reciprocalcogecontroldichroismdirectionaldomainsin-situ
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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Non-reciprocal directional dichroism, also called the optical-diode effect, is an appealing functional property inherent to the large class of non-centrosymmetric magnets. However, the in-situ electric control of this phenomenon is challenging as it requires a set of conditions to be fulfilled: Special symmetries of the magnetic ground state, spin-excitations with comparable magnetic- and electric-dipole activity and switchable electric polarization. We demonstrate the isothermal electric switch between domains of Ba$_2$CoGe$_2$O$_7$ possessing opposite magnetoelectric susceptibilities. Combining THz spectroscopy and multiboson spin-wave analysis, we show that unbalancing the population of antiferromagnetic domains generates the non-reciprocal light absorption of spin excitations.

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