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arxiv 2212.05278 v3 pith:U3IH7NCX submitted 2022-12-10 cond-mat.str-el cond-mat.other

Ring-Exchange Interaction Effects on Magnons in Dirac Magnet CoTiO₃

classification cond-mat.str-el cond-mat.other
keywords magnonmodelcotiodeterminediracflavorinteractioninteractions
verification ladder T0 review T1 audit T2 compute T3 formal T4 reserved
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The magnetic interactions that determine magnetic order and magnon energies typically involve only two spins. While rare, multi-spin interactions can also appear in quantum magnets and be the driving force in the ground state selection and in the nature of its excitations. By performing time-domain terahertz and magneto-Raman spectroscopy measurements combined with theoretical modeling, we determine the origin of the magnon excitation gap in Dirac antiferromagnet CoTiO$_3$. By adding a ring-exchange interaction in a hexagonal plaquette of the honeycomb lattice to both an XXZ spin model and to a low energy spin-orbital flavor wave model, a gap is generated in the magnon spectrum at the Brillouin zone center. With this addition, the flavor wave model reproduces a large swath of experimental results including terahertz, Raman, inelastic neutron scattering, and magnetization experiments.

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