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arxiv: 2505.04868 · v1 · pith:UVORZ5Q6new · submitted 2025-05-08 · ❄️ cond-mat.str-el

Ground-states of the Shastry-Sutherland Lattice Materials Gd₂Be₂GeO₇ and Dy₂Be₂GeO₇

classification ❄️ cond-mat.str-el
keywords materialsmelilitesshastry-sutherlandlatticelikelymagneticmagnetizationrare-earth
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The recent realization that the rare-earth melilites RE$_2$Be$_2$GeO$_7$ host the Shastry-Sutherland lattice within planes of RE$^{3+}$ ions has sparked a number of studies. This family of materials lacks appreciable site mixing and conductivity, making them promising candidates for the Shastry-Sutherland model. Herein, we present the magnetic ground states of two of these rare-earth melilites: RE = Gd and Dy. We find, through measurements of magnetic susceptibility, magnetization, and specific heat capacity (RE = Dy only), that these two melilites are antiferromagnets (T$_N$ $\sim$~1~K). Gd$_2$Be$_2$GeO$_7$, in accordance with its electronic configuration, has isotropic single-ion anisotropy but shows a quadratic contribution to its magnetization. Dy$_2$Be$_2$GeO$_7$ has Ising-like single-ion ansiotropy and is likely an effective spin-$1/2$ system. Both materials exhibit metamagnetic transitions. We identify this transition in Dy$_2$Be$_2$GeO$_7$, occurring at 86(1)~mT for T=500~mK, to likely be a spin-flip transition.

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  1. Spiral and Mixed Plaquette-Dimer Phases in the $S=1$ and $3/2$ Shastry-Sutherland Heisenberg Model

    cond-mat.str-el 2026-05 unverdicted novelty 5.0

    DMRG and CMFT calculations reveal intermediate spiral and mixed plaquette-dimer phases for S=1 and S=3/2 on the Shastry-Sutherland lattice, with a global S-g phase diagram constructed from known limits.