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arxiv: 1508.07841 · v1 · pith:XQN2ROB2new · submitted 2015-08-31 · ❄️ cond-mat.str-el · cond-mat.mtrl-sci

Formation and observation of a quasi-two-dimensional d_(xy) electron liquid in epitaxially stabilized Sr_(2-x)La_(x)TiO₄ thin films

classification ❄️ cond-mat.str-el cond-mat.mtrl-sci
keywords srtioelectronenergyformationinterfacelaaloliquidobservation
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We report the formation and observation of an electron liquid in Sr$_{2-x}$La$_{x}$TiO$_4$, the quasi-two-dimensional counterpart of SrTiO$_3$, through reactive molecular-beam epitaxy and {\it in situ} angle-resolved photoemission spectroscopy. The lowest lying states are found to be comprised of Ti 3$d_{xy}$ orbitals, analogous to the LaAlO$_3$/SrTiO$_3$ interface and exhibit unusually broad features characterized by quantized energy levels and a reduced Luttinger volume. Using model calculations, we explain these characteristics through an interplay of disorder and electron-phonon coupling acting co-operatively at similar energy scales, which provides a possible mechanism for explaining the low free carrier concentrations observed at various oxide heterostructures such as the LaAlO$_3$/SrTiO$_3$ interface.

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