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Gapless spin-liquid state in the structurally disorder-free triangular antiferromagnet NaYbO$_2$

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arxiv 1901.07810 v1 pith:ZYID4R63 submitted 2019-01-23 cond-mat.str-el cond-mat.mtrl-sci

classification cond-mat.str-elcond-mat.mtrl-sci
keywords naybospin-liquidtriangularantiferromagnetgaplesslow-temperaturemagneticphase
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abstract

We present the structural characterization and low-temperature magnetism of the triangular-lattice delafossite NaYbO$_2$. Synchrotron x-ray diffraction and neutron scattering exclude both structural disorder and crystal-electric-field randomness, whereas heat-capacity measurements and muon spectroscopy reveal the absence of magnetic order and persistent spin dynamics down to at least 70\,mK. Continuous magnetic excitations with the low-energy spectral weight accumulating at the $K$-point of the Brillouin zone indicate the formation of a novel spin-liquid phase in a triangular antiferromagnet. This phase is gapless and shows a non-trivial evolution of the low-temperature specific heat. Our work demonstrates that NaYbO$_2$ practically gives the most direct experimental access to the spin-liquid physics of triangular antiferromagnets.

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  1. Single-site magnetic anisotropy governed by inter-layer cation charge imbalance in triangular-lattice AYbX$_2$

    cond-mat.str-el 2019-09 conditional novelty 6.0 of 10

    The strongly anisotropic g factors of Yb3+ in NaYbS2 and NaYbO2 are controlled mainly by the charge contrast between in-plane Yb3+ neighbors and inter-layer Na+ ions, with a more homogeneous cation environment yieldin...

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