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A New Method of Measuring 81Kr and 85Kr Abundances in Environmental Samples
Atomic Physics · Submitted 25 Nov 2003
abstract compiled · 2026-09-23 · no language-model review
The authors' main claim We demonstrate a new method for determining the 81Kr/Kr ratio in environmental samples based upon two measurements: the 85Kr/81Kr ratio measured by Atom Trap Trace Analysis (ATTA) and the 85Kr/Kr ratio measured by Low-Level Counting (LLC).
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The abstract, sentence by sentence
We demonstrate a new method for determining the 81Kr/Kr ratio in environmental samples based upon two measurements: the 85Kr/81Kr ratio measured by Atom Trap Trace Analysis (ATTA) and the 85Kr/Kr ratio measured by Low-Level Counting (LLC). This method can be used to determine the mean residence time of groundwater in the range of 10^5 - 10^6 a. It requires a sample of 100 micro-l STP of Kr extracted from approximately two tons of water. With modern atmospheric Kr samples, we demonstrate that the ratios measured by ATTA and LLC are directly proportional to each other within the measurement error of +/- 10%; we calibrate the 81Kr/Kr ratio of modern air measured using this method; and we show that the 81Kr/Kr ratios of samples extracted from air before and after the development of the nuclear industry are identical within the measurement error.
background contribution method result interpretation main claim
| # | sentence | role | the authors' own work | states the main conclusion | strength |
|---|---|---|---|---|---|
| s0 | We demonstrate a new method for determining the 81Kr/Kr ratio in environmental samples based upon two measurements: the 85Kr/81Kr ratio measured by Atom Trap Trace Analysis (ATTA) and the 85Kr/Kr ratio measured by Low-Level Counting (LLC). | contribution 0.60 | 0.93 | 0.43 | asserted 1.00 |
| s1 | This method can be used to determine the mean residence time of groundwater in the range of 10^5 - 10^6 a. | contribution 0.54 | 0.60 | 0.27 | hedged possibility 0.52 |
| s2 | It requires a sample of 100 micro-l STP of Kr extracted from approximately two tons of water. | method 0.89 | 0.60 | 0.04 | asserted 1.00 |
| s3 | With modern atmospheric Kr samples, we demonstrate that the ratios measured by ATTA and LLC are directly proportional to each other within the measurement error of +/- 10%; we calibrate the 81Kr/Kr ratio of modern air measured using this method; and we show that the 81Kr/Kr ratios of samples extracted from air before and after the development of the nuclear industry are identical within the measurement error. | result 0.98 | 0.96 | 0.33 | asserted 1.00 |
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The paper
Original abstract
We demonstrate a new method for determining the 81Kr/Kr ratio in environmental samples based upon two measurements: the 85Kr/81Kr ratio measured by Atom Trap Trace Analysis (ATTA) and the 85Kr/Kr ratio measured by Low-Level Counting (LLC). This method can be used to determine the mean residence time of groundwater in the range of 10^5 - 10^6 a. It requires a sample of 100 micro-l STP of Kr extracted from approximately two tons of water. With modern atmospheric Kr samples, we demonstrate that the ratios measured by ATTA and LLC are directly proportional to each other within the measurement error of +/- 10%; we calibrate the 81Kr/Kr ratio of modern air measured using this method; and we show that the 81Kr/Kr ratios of samples extracted from air before and after the development of the nuclear industry are identical within the measurement error.
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How the literature uses it
2 arXiv papers cite this in 3 sentences
Papers citing it · 1 sentence without a confident label
Uses its data or values 2 papers
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The present-day activity concentration is approximately 1.4 [ref] , corresponding to a relative isotopic abundance of 85/nat of 2e-11 [ref] .
Krypton assay in xenon at the ppq level using a gas chromatographic system and mass spectrometer · Introduction · 0.93
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This number roughly corresponds to a relative isotopic abundance of [85]Kr/[nat]Kr = 2e-11 [ref] .
Intrinsic backgrounds from Rn and Kr in the XENON100 experiment · Krypton · 0.87
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