A reaction-field model with no fitted Hamiltonian parameters reproduces the magnetic excitation spectrum of Ho3Ga5O12 and attributes its magnetic ordering to nuclear hyperfine coupling.
Crystal fields and magnetic structure of the Ising antiferromagnet Er$_3$Ga$_5$O$_{12}$
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abstract
Rare earth garnets are an exciting playground for studying the exotic magnetic properties of the frustrated hyperkagome lattice. Here we present a comprehensive study of the single ion and collective magnetic properties of the garnet Er$_3$Ga$_5$O$_{12}$. Using inelastic neutron scattering, we find a crystal field ground state doublet for Er$^{3+}$ with strong Ising anisotropy along local [100] axes. Magnetic susceptibility and heat capacity measurements provide evidence for long-range magnetic ordering with $T_N$~$=$~0.8~K, and no evidence for residual entropy is found when cooling through the ordering transition. Neutron powder diffraction reveals that the ground state spin configuration corresponds to the six-sublattice, Ising antiferromagnetic state ($\Gamma_3$) common to many of the rare earth garnets. However, we also found that $\mu$SR appears to be insensitive to the ordering transition in this material, in which a low-temperature relaxation plateau was observed with no evidence of spontaneous muon precession. The combined muon and neutron results may be indicative of a dynamical ground state with a relatively long correlation time. Despite this potential complication, our work indicates that Er$_3$Ga$_5$O$_{12}$ is an excellent model system for studying the complex metamagnetism expected for a multi-axis antiferromagnet.
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Modeling Spin Dynamics in the Singlet Ground State Garnet Ho3Ga5O12
A reaction-field model with no fitted Hamiltonian parameters reproduces the magnetic excitation spectrum of Ho3Ga5O12 and attributes its magnetic ordering to nuclear hyperfine coupling.