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Crystal fields and magnetic structure of the Ising antiferromagnet Er$_3$Ga$_5$O$_{12}$

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arxiv 1905.03687 v2 pith:QUPKUSQL submitted 2019-05-09 cond-mat.str-el

classification cond-mat.str-el
keywords magneticstateevidencegroundisingneutronorderingantiferromagnet
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abstract

Rare earth garnets are an exciting playground for studying the exotic magnetic properties of the frustrated hyperkagome lattice. Here we present a comprehensive study of the single ion and collective magnetic properties of the garnet Er$_3$Ga$_5$O$_{12}$. Using inelastic neutron scattering, we find a crystal field ground state doublet for Er$^{3+}$ with strong Ising anisotropy along local [100] axes. Magnetic susceptibility and heat capacity measurements provide evidence for long-range magnetic ordering with $T_N$~$=$~0.8~K, and no evidence for residual entropy is found when cooling through the ordering transition. Neutron powder diffraction reveals that the ground state spin configuration corresponds to the six-sublattice, Ising antiferromagnetic state ($\Gamma_3$) common to many of the rare earth garnets. However, we also found that $\mu$SR appears to be insensitive to the ordering transition in this material, in which a low-temperature relaxation plateau was observed with no evidence of spontaneous muon precession. The combined muon and neutron results may be indicative of a dynamical ground state with a relatively long correlation time. Despite this potential complication, our work indicates that Er$_3$Ga$_5$O$_{12}$ is an excellent model system for studying the complex metamagnetism expected for a multi-axis antiferromagnet.

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Reviewed papers in the Pith corpus that reference this work. Sorted by Pith novelty score. Full citation record

  1. Modeling Spin Dynamics in the Singlet Ground State Garnet Ho3Ga5O12

    cond-mat.str-el 2019-08 conditional novelty 6.0 of 10

    A reaction-field model with no fitted Hamiltonian parameters reproduces the magnetic excitation spectrum of Ho3Ga5O12 and attributes its magnetic ordering to nuclear hyperfine coupling.

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