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arxiv: 1009.0553 · v3 · pith:BVYO6V2Mnew · submitted 2010-09-02 · ❄️ cond-mat.mes-hall · cond-mat.mtrl-sci

Resonance energy transfer near metal nanostructures mediated by surface plasmons

classification ❄️ cond-mat.mes-hall cond-mat.mtrl-sci
keywords transfernearenergymoleculesmetalresonancebalancecalculations
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We develop a unified theory of plasmon-assisted resonance energy transfer (RET) between molecules near a metal nanostructure that maintains energy balance between transfer, dissipation, and radiation. We show that in a wide range of parameters, including in the near field, RET is dominated by plasmon-enhanced radiative transfer (PERT) rather than by a nonradiative transfer mechanism. Our numerical calculations performed for molecules near the Ag nanoparticle indicate that RET magnitude is highly sensitive to molecules' positions.

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