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arxiv: 1307.8378 · v2 · pith:ZKP4EQCLnew · submitted 2013-07-31 · ❄️ cond-mat.mes-hall · quant-ph

Non-markovian polariton dynamics in organic strong coupling

classification ❄️ cond-mat.mes-hall quant-ph
keywords organicpolaritonstatecoupleddynamicslifetimelowernon-markovian
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Strongly coupled organic systems are characterized by unusually large Rabi splittings, even in the vacuum state. They show the counter-intuitive feature of a lifetime of the lower polariton state longer than for all other excited states. Here we build up a new theoretical framework to understand the dynamics of such coupled system. In particular, we show that the non-Markovian character of the relaxation of the dressed organic system explains the long lifetime of the lower polariton state.

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